Origin of the Broad Lifetime Distribution of Localized Excitons in InGaN/GaN Quantum Dots

نویسندگان

  • M. Winkelnkemper
  • M. Dworzak
  • T. P. Bartel
  • A. Strittmatter
  • A. Hoffmann
  • D. Bimberg
چکیده

We derive an energy-dependent decay-time distribution function from the multi-exponential decay of the ensemble photoluminescence (PL) of InxGa1-xN/GaN quantum dots (QDs), which agrees well with recently published singleQD time-resolved PL measurements. Using eight-band k·p modelling, we show that the built-in piezoand pyroelectric fields within the QDs cause a sensitive dependence of the radiative lifetimes on the exact QD geometry and composition. Moreover, the radiative lifetimes also depend heavily on the composition of the direct surrounding of the QDs. A broad lifetime distribution occurs even for moderate variations of the QD structure. Thus, for unscreened fields a multi-exponential decay of the ensemble PL is generally expected in this material system. (accepted at Physica Status Solidi (b). c ©2008 WILEY-VCH)

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تاریخ انتشار 2008